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By Ralph E. White, John O'M. Bockris, Brian E. Conway (Eds.)

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Extra resources for Modern Aspects of Electrochemistry, Vol. 33

Example text

Of Eq. " Equation (32) suffers from the same shortcomings as Eq. (27). In particular, a@/aTmust be known independently for the same metal sample as the one used as an electrode. Moreover, in view of the crystal-face specificity of End, its temperature coefficient is also expected to depend on the crystallographic orientation. Being a differential quantity, aE,JaT is an even more delicate experimental quantity than Enlo itself. o~ the basis of a simple up-and-down molecular model for water," this positive value has been taken to indicate a preferential orientation, with the negative end of the molecular dipole (oxygen) toward the metal surface.

Equation (32) suffers from the same shortcomings as Eq. (27). In particular, a@/aTmust be known independently for the same metal sample as the one used as an electrode. Moreover, in view of the crystal-face specificity of End, its temperature coefficient is also expected to depend on the crystallographic orientation. Being a differential quantity, aE,JaT is an even more delicate experimental quantity than Enlo itself. o~ the basis of a simple up-and-down molecular model for water," this positive value has been taken to indicate a preferential orientation, with the negative end of the molecular dipole (oxygen) toward the metal surface.

35)with Eq. (34) gives Equation (36) shows that information on gs(dip) can be obtained only if = b~ and f(dip) = 0 or is precisely known. Both cases are difficult to meet. df n e Potential of Zero Charge Figure 7. Adswon of tm ekcmnegarive w e s from tbe gas phase onto a su&e genea dipolar layer due to e l m m&~~metalto~~Adsorptionofsnions~~ elear& simalates the s i t d o n when the p d v e charge on the metal cmpma for the dmkd negative charge (madiffuselayer charge), and not when the charge rm the metal is m.

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